World Environment and Energy (2011)
 

Non-fossil natural gas

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Although fossil natural gas is an important source of greenhouse gases, emitting 40−50 million tonnes per year, virtually all anthropogenic, it is not the largest source of methane, either natural or man-made. The following table are estimates of annual emissions of methane from various sources, in millions of tonnes.

Source Natural Man-made
Natural Wetlands 100-200  
Rice paddies   25-170
Ruminants 45-80 25-40
Fossil NG   40-50
Biomass burning 10-30 10-50
Termites 10-100  
Landfills & compost   20-70

Obviously, the ranges for some of these sources are very high, but if we add up the means for each, we get the following situation:

  Natural Man-made
Mean 288 250

It is therefore clear that man is contributing nearly as much as nature. In fact, he is emitting more than nature because he has reduced the emissions from natural wetlands by marsh drainage. This is evidenced by the fact that the methane content of the atmosphere has increased 225 per cent, from 800 ppbv (1850) to 1800 ppbv (2000). It is evident that this increase is due to human activities, such as increased areas of rice farming, increased cattle farming and, of course, using fossil-fuel NG. This makes a significant difference to climate-change.

A recent worry has been that, over the centuries, natural gas has been generated in vast quantities in peat bogs in tundra areas. This has been prevented from escaping by a thick layer of ice or permafrost on the surface. The permafrost thickness varies from a few tens of cm to over 1,000 m. In the same was as the polar ice caps are melting because of climate change, so the permafrost is also melting and, in doing so, releases the imprisoned natural gas. The quantity thus released can be very significant and can be responsible for an important increase in atmospheric greenhouse gases. This is obviously a very serious positive feedback effect, because this will cause a further increase in temperature, melting even more permafrost. The quantity of methane captured in the permafrost is not known with accuracy.

Another potential problem may be with methane hydrates or clathrates. Under given temperature and pressure conditions, methane (and carbon dioxide) will form a clathrate which consists of a lattice of water molecules capturing a gas molecule to form a crystalline solid, in an unstable state. Under suitable conditions, decomposing seaweed or other vegetable matter, falling to the bottom , produces methane and carbon dioxide that can be captured. It is also surmised that "leaking" gases from fossil sources may produce clathrates. These conditions are optimised in medium-depth seas or lakes with an abundance of living matter, such as the Gulf of Mexico or some tropical lakes. The quantity of methane held in clathrates is unknown but accumulation over millennia means that it is in millions of tonnes. As long as it remains at the bottom, there is no problem. The problem starts when the conditions cause the clathrate crystal to disintegrate, releasing the gas. This may be caused by a change of temperature or pressure or even a mechanical shock; the drama can occur because the shock of disintegration of one crystal can cause a neighbouring crystal to disintegrate, in turn, and a physical chain reaction can result, releasing enormous quantities of gases. This has happened on rare occasions and is fairly speculative. It should be noted that the Lake Nyos disaster in 1986 was probably not due to a massive clathrate disintegration; the current theory is that large volumes of carbon dioxide, from volcanic activity, super-saturated in the water, was suddenly released.